Piezo-Transmissive Structure Using a Multi-layered Heterogeneous Film for Optical Transmittance Modulation

ACS Appl Mater Interfaces. 2023 Apr 26;15(16):20531-20540. doi: 10.1021/acsami.3c01619. Epub 2023 Apr 13.

Abstract

As the damage caused by the recent climate crisis increases, efforts are being made to develop low-power and high-efficiency technologies to reduce pollution for energy production worldwide. Among them, research on the mechano-responsive optical transmittance modulation technology is being actively conducted as it can be applied to various application fields for reducing energy consumption: low-power sensors and smart windows. The piezo-transmittance structure, which is one of the optical transmittance modulation structures, has fewer constraints on the installation environment; therefore, many applications have been proposed. However, it is still challenging to fabricate a piezo-transmittance structure with a large-area production, high throughput, and good tunability because of complex curing and dissolution processes. Herein, we present an efficient fabrication method for a multi-layered piezo-transmittance structure using a large-area abrasive mold and thermal imprinting process. The piezo-transmittance performance (e.g., sensitivity and relative change of transmittance) shows temperature/humidity-independent characteristics and can be designed by tuning design parameters such as the number of layers, abrasive grade, and film material. Also, the surrogate model of the performance obtained from the Monte Carlo simulation and prediction model can offer tunability for various applications. Finally, we demonstrated two energy-efficient applications: the smart window integrated with a hydraulic pump showed high thermal efficiency in indoor environment control, and the telemetry system was demonstrated to measure pressure remotely.

Keywords: abrasive; multi-layered structure; piezo-transmittance; smart window; telemetry; thermal imprinting.