Dual electro- and magneto-induced bending actuators of magnetite-loaded agarose ionogels

Carbohydr Polym. 2023 Jun 15:310:120741. doi: 10.1016/j.carbpol.2023.120741. Epub 2023 Feb 23.

Abstract

Magnetic ionogels are a new kind of gel composites which combine the elastic properties from the swollen gel matrix and the magnetic properties from a magnetic filler. The dual electro-magneto-responsive agarose ionogels (AG IGels) were fabricated by a solution casting method using 1-butyl-3-methylimidazolium chloride [Bmim][Cl] as the ionic liquid solvent, and embedded with magnetite nanoparticles (Fe3O4 NPs). The addition of Fe3O4 NPs induced the high bending responses under applied electric and magnetic fields via the electronic polarization and magnetic interaction. The 3.0 wt.% Fe3O4/AG MagIGel showed the largest deflection distances relative to other magnetic gel composites; 14.92, 8.96, and 21.63 mm under the applied electric fields of 600 V/mm in silicone oil, 60 V/mm in air, and under the applied magnetic field of 600 G in air, respectively. The bending distances were of comparable in magnitudes to other electro-magneto-responsive materials. Thus, the fabricated Fe3O4/AG MagIGels are demonstrated here as potential for soft electric-magnetic actuator applications.

Keywords: Actuator; Agarose; Bending responses; Ionic liquid; Magnetic gel; Magnetite.