Spatially structured quantum states, such as orbital angular momentum (OAM) squeezing and entanglement, is currently a popular topic in quantum optics. The method of generating and manipulating spatial quantum states on demand needs to be explored. In this paper, we generated OAM mode squeezed states of -5.4 dB for the L G0+1 mode and -5.3 dB for the L G0-1 mode directly by an optical parametric oscillator (OPO) for the first time. Additionally, we demonstrated that the OAM mode squeezed and entangled states were respectively generated by manipulating the nonlinear process of the OPO by controlling the relative phase of two beams of different modes, thus making two different spatial multimode pump beams. We characterized the Laguerre-Gaussian (LG) entangled states by indirectly measuring the squeezing for the H G 10(45∘) mode and H G 10(135∘) mode, and directly measuring the entanglement between the L G0+1 and L G0-1 modes. The effective manipulation of the OAM quantum state provides a novel insight into the continuous variable quantum state generation and construction on demand for high-dimensional quantum information and quantum metrology.