A new strategy for risk assessment of PM2.5-bound elements by considering the influence of wind regimes

Jéssica Caroline Dos Santos-Silva; Sanja Potgieter-Vermaak; Sandra Helena Westrupp Medeiros; Luiz Vitor da Silva; Danielli Ventura Ferreira; Camila Ariele Bufato Moreira; Priscila Caroline de Souza Zorzenão; Theotonio Pauliquevis; Ana Flávia Locateli Godoi; Rodrigo Augusto Ferreira de Souza; Carlos Itsuo Yamamoto; Ricardo Henrique Moreton Godoi

doi:10.1016/j.scitotenv.2023.162131

A new strategy for risk assessment of PM_2.5-bound elements by considering the influence of wind regimes

Sci Total Environ. 2023 May 10:872:162131. doi: 10.1016/j.scitotenv.2023.162131. Epub 2023 Feb 10.

Authors

Affiliations

¹ Postgraduate Program in Water Resources and Environmental Engineering, Federal University of Paraná, Curitiba, Paraná, Brazil.
² Ecology & Environment Research Centre, Department of Natural Science, Manchester Metropolitan University, Manchester M1 5GD, United Kingdom; Molecular Science Institute, University of the Witwatersrand, Johannesburg, South Africa.
³ Department of Environmental and Sanitary Engineering, University of the Region of Joinville, Joinville, Santa Catarina, Brazil.
⁴ Department of Environmental Engineering, Federal University of Paraná, Curitiba, Paraná, Brazil.
⁵ Department of Chemical Engineering, Federal University of Paraná, Curitiba, Paraná, Brazil.
⁶ Department of Environmental Sciences, Federal University of São Paulo, Diadema, São Paulo, Brazil.
⁷ School of Technology, Amazonas State University, Manaus, Amazonas, Brazil.
⁸ Postgraduate Program in Water Resources and Environmental Engineering, Federal University of Paraná, Curitiba, Paraná, Brazil; Department of Environmental Engineering, Federal University of Paraná, Curitiba, Paraná, Brazil. Electronic address: rhmgodoi@ufpr.br.

PMID: 36773898
DOI: 10.1016/j.scitotenv.2023.162131

Abstract

For regulatory purposes, air pollution has been reduced to management of air quality control regions (AQCR), by inventorying pollution sources and identifying the receptors significantly affected. However, beyond being source-dependent, particulate matter can be physically and chemically altered by factors and elements of climate during transport, as they act as local environmental constraints, indirectly modulating the adverse effects of particles on the environment and human health. This case study, at an industrial site in a Brazilian coastal city - Joinville, combines different methodologies to integrate atmospheric dynamics in a strategic risk assessment approach whereby the influence of different wind regimes on environmental and health risks of exposure to PM_2.5-bound elements, are analysed. Although Joinville AQCR has been prone to stagnation/recirculation events, distinctly different horizontal wind circulation patterns indicate two airsheds within the region. The two sampling sites mirrored these two conditions and as a result we report different PM_2.5 mass concentrations, chemical profiles, geo-accumulation, and ecological and human health risks. In addition, feedback mechanisms between the airsheds seem to aggravate the air quality and its effects even under good ventilation conditions. Recognizably, the risks associated with Co, Pb, Cu, Ni, Mn, and Zn loadings were extremely high for the environment as well as being the main contributors to elevated non-carcinogenic risks. Meanwhile, higher carcinogenic risks occurred during stagnation/recirculation conditions, with Cr as the major threat. These results highlight the importance of integrating local airshed characteristics into the risk assessment of PM_2.5-bound elements since they can aggravate air pollution leading to different risks at a granular scale. This new approach to risk assessment can be employed in any city's longer-term development plan since it provides public authorities with a strategic perspective on incorporating environmental constraints into urban growth planning and development zoning regulations.

Keywords: Development zoning; Health risks; Heavy metals; Meteorological conditions; PM(2.5).