A new method for measuring magnetorheological fluid redispersibility by testing yield stresses of sediments at different depths

Rev Sci Instrum. 2023 Jan 1;94(1):015103. doi: 10.1063/5.0129497.

Abstract

Magnetorheological fluid (MRF) is a widely used smart material that suffers from sedimentation. Since sedimentation is unavoidable, it is crucial to study and improve the redispersibility of MRFs. However, previous redispersibility testing methods have problems, such as complicated operation and low precision. Simultaneously, a simple and effective method is urgently needed for high-precision modeling of MRF sedimentation to test the rheological properties of settled MRFs at different depths. After systematically analyzing the redispersion problem, this paper proposes decoupling the energy required for redispersing settled MRFs into two parts, which are related to different factors. These two parts are the energy required to separate the agglomerated particles (related to the MRF formula) and that to redisperse the settled MRF uniformly vertically against gravity (related to the solid concentration and packing limit). The energy that separates the agglomerated particles is proportional to the shear stress of slowly shearing the corresponding agglomerated samples, i.e., the yield stress. Thus, this paper proposes a simple microdamage quasi-static indentation method to measure the yield stresses of settled MRFs at different depths to characterize the redispersibility of the corresponding MRFs. Herein, this method is applied to study the mechanisms of the influences of surfactants, thixotropic agents, and their networks on the redispersibility of MRFs. The results indicate that a well-dispersed plate-like thixotropic agent network can effectively improve redispersibility, while surfactants with poor compatibility degrade redispersibility. In summary, this redispersibility test method will greatly facilitate studies of MRFs, such as optimizing the formulas and establishing sedimentation models.