Water treatment consumes lots of energy from fossil fuels nowadays, and the emission of CO2 enhances the temperature on earth, resulting in more and more hazards. Thus, clean water production enabled by green energy without CO2 emission is attracting more and more attention. Herein, we propose a novel solar evaporation system achieving both solar evaporation and water storage with two different unique hydrogels based on a three-dimensional (3D) printing technique. The hydrogel absorber demonstrates an ultrahigh absorptance (98.2%) of solar light, while the water-storage hydrogel absorbs more than 100 times its own weight of water, demonstrating super water-storage performance with strong self-adhesiveness. The solar vapor generation rate can be as high as 3.14 kg·m-2·h-1, with a solar evaporation efficiency up to 91.2% irradiated by 1.43 sun. Furthermore, our environmentally friendly solar evaporation system achieves ultrahigh water purification efficiency of 99.99% for salt, heavy ions, and acid/alkaline with remarkable stability and durability. Our solar evaporation system promises long-lasting applications for the hydrological cycle enabled by solar energy, such as seawater desalination, sterilization, wastewater purification, and so on.
Keywords: hydrogel; hydrological cycle; self-adhesiveness; solar evaporation system; super water-storage performance.