Sources of Variability in Real-time Monitoring Data for Fine Particulate Matter: Comparability of Three Wearable Monitors in an Urban Setting

Environ Sci Technol Lett. 2019 Apr 9;6(4):222-227. doi: 10.1021/acs.estlett.9b00115. Epub 2019 Mar 18.

Abstract

The increasing availability of portable air pollution monitoring devices has greatly enhanced the ability to measure personal exposures in real time. However, these devices vary considerably in their cost and specifications, and questions remain as to their reliability and practicality for use in epidemiological investigations. In this field study, three personal PM2.5 exposure monitors (two nephelometers, one optical particle counter) were compared in an urban setting to assess their feasibility for use in future studies. In total, 3963 1-min measurements were collected over 12 days from locations of several types (e.g., above and below-ground subway stations, sidewalks next to urban traffic, outdoor construction sites) in the Washington, D.C. metropolitan area. Overall, we observed moderate-to-high agreement in pairwise comparisons of PM2.5 concentrations between devices (R2 range: 0.37 to 0.75). Bland-Altman plots showed that differences in device agreement varied over the range of mean concentrations. In linear mixed models adjusting for temperature and relative humidity, we saw significant interaction between device and location (p<0.05), suggesting that the relationship between devices was not constant in all locations. Our finding of heterogeneity in instrument comparability by location may have important implications in epidemiologic studies incorporating personal PM2.5 measurements.

Keywords: PM2.5; ambient monitoring; personal exposure.