Double-Cavity Modulation of Exciton Polaritons in CsPbBr3 Microwire

Nano Lett. 2022 Dec 14;22(23):9365-9371. doi: 10.1021/acs.nanolett.2c03147. Epub 2022 Nov 18.

Abstract

The lead halide perovskite has become a promising candidate for the study of exciton polaritons due to their excellent optical properties. Here, both experimental and simulated results confirm the existence of two kinds of Fabry-Pérot microcavities in a single CsPbBr3 microwire with an isosceles right triangle cross section, and we experimentally demonstrate that confined photons in a straight and a folded Fabry-Pérot microcavity are strongly coupled with excitons to form exciton polaritons. Furthermore, we reveal the polarization characteristic and double-cavity modulation of exciton polaritons emission by polarization-resolved fluorescence spectroscopy. Our results not only prove that the modulation of exciton polaritons emission can occur in this simple double-cavity system but also provide a possibility to develop related polariton devices.

Keywords: CsPbBr3 microwire; double Fabry−Pérot microcavity; exciton polaritons; polarization anisotropy.