Natural gels and biomimetic hydrogel materials have been able to achieve outstanding integrated mechanical properties due to the gain of natural biological structures. However, nearly every natural biological structure relies on water as solvents or carriers, which limits the possibility in extreme conditions, such as sub-zero temperatures and long-term application. Here, peptide-enhanced eutectic gels were synthesized by introducing α-helical "molecular spring" structure into deep eutectic solvent. The gel takes full advantage of the α-helical structure, achieving high tensile/compression, good resilience, superior fracture toughness, excellent fatigue resistance and strong adhesion, while it also inherits the benefits of the deep eutectic solvent and solves the problems of solvent volatilization and freezing. This enables unprecedentedly long and stable sensing of human motion or mechanical movement. The electrical signal shows almost no drift even after 10,000 deformations for 29 hours or in the -20 °C to 80 °C temperature range.
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