The use of plastic scintillation microspheres in flow scintillation analysis

Abstract

This manuscript deals with the possible utilization of plastic microspheres for radiation detection. The aim was to determine the suitability of microspheres for this application, factors that affect detection efficiency, and based on the evaluation of current state technology to design and test a constructional solution suitable for this use. Three detection cell variations and their configurations, which utilize plastic microspheres, were tested for their response to selected militarily important radionuclides during a series of static measurements. Based on the results of static measurements, the most structurally suitable cell variation was subsequently tested for flow scintillation analysis. Among the cells designed for flow scintillation counting in 2π geometry, the highest achieved detection efficiency for 241Am was 13.1 ± 0.7% using Cell #5, for 90Sr/Y was 71.2 ± 3.9% using Cell #10 and for 3H was 3.9 ± 0.2% using Cell #5 respectively. Cell #10 was evaluated to perform universally the best despite achieving slightly lower detection efficiencies for 241Am and 3H than Cell #5, as the results were easily replicable and due to the cell constructional simplicity, its application was problem-free.

Keywords: Detection cell; Flow scintillation analysis; Fluorescence; Plastic microspheres; Plastic scintillation; Scintillation capillary.