Highly Active and Thermally Robust Nickel Enolate Catalysts for the Synthesis of Ethylene-Acrylate Copolymers

Angew Chem Int Ed Engl. 2022 Aug 26;61(35):e202206637. doi: 10.1002/anie.202206637. Epub 2022 Jul 18.

Abstract

The insertion copolymerization of polar olefins and ethylene remains a significant challenge in part due to catalysts' low activity and poor thermal stability. Herein we demonstrate a strategy toward addressing these obstacles through ligand design. Neutral nickel phosphine enolate catalysts with large phosphine substituents reaching the axial positions of Ni achieve activity of up to 7.7×103 kg mol-1 h-1 (efficiency >35×103 g copolymer/g Ni) at 110 °C, notable for ethylene/acrylate copolymerization. NMR analysis of resulting copolymers reveals highly linear microstructures with main-chain ester functionality. Structure-performance studies indicate a strong correlation between axial steric hindrance and catalyst performance.

Keywords: Acrylate; Catalysis; Copolymers; Nickel; Olefins.

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