Photoemission of Plasmonic Gold Nanostars in Laser-Controlled Electron Current Devices for Technical and Biomedical Applications

Sensors (Basel). 2022 May 29;22(11):4127. doi: 10.3390/s22114127.

Abstract

The main goal of this work was to modify the previously developed blade-type planar structure using plasmonic gold nanostars in order to stimulate photofield emission and provide efficient laser control of the electron current. Localization and enhancement of the field at the tips of gold nanostars provided a significant increase in the tunneling electron current in the experimental sample (both electrical field and photofield emission). Irradiation at a wavelength in the vicinity of the plasmon resonance (red laser) provided a gain in the photoresponse value of up to 5 times compared to irradiation far from the resonance (green laser). The prospects for transition to regimes of structure irradiation by femtosecond laser pulses at the wavelength of surface plasmon resonance, which lead to an increase in the local optical field, are discussed. The kinetics of the energy density of photoinduced hot and thermalized electrons is estimated. The proposed laser-controlled matrix current source is promising for use in X-ray computed tomography systems.

Keywords: X-ray biosensor; diamond-like carbon; electron temperature; gold nanostar; hot electron; photoinduced electron emission; surface plasmon resonance.

MeSH terms

  • Electrons
  • Gold* / chemistry
  • Lasers
  • Metal Nanoparticles* / chemistry
  • Surface Plasmon Resonance / methods

Substances

  • Gold