Although children have been identified as a vulnerable group highly susceptible to traffic-related air pollution, their exposure during school commutes to traffic-related pollutants and the relevant health impact is rarely studied. In this study, we measured black carbon (BC) and particulate matter (PM: PM1, PM2.5, and PM10) concentrations that children are exposed to during their multi-modal (walking, private cars, and e-bikes) commuting trips to schools in Xi'an, China. A multi-parameter inhalation rate assessment model was developed in combination with the Multi-Path Particle Dosimetry (MPPD) model to quantify the deposition dose in different parts of children's respiratory system (head, tracheobronchial (TB), pulmonary (PUL)). Results show that walking to school exposed children to the lowest PM1, PM2.5, and BC concentrations, whereas riding an e-bike led to significantly elevated exposure to PM1 and BC than the other two modes. This is due to children's closer proximity to vehicle tail pipe emissions when they bike to school on road or roadside. The PM and BC concentrations showed remarkable increases in comparison to background concentrations during children's school commutes. Urban background (UB) concentration, traffic volume (TV), time of day, and meteorological parameters could influence a child's personal exposure, and the impact of each factor vary across different transportation modes. Particle size of the pollutant affects its deposition site in the respiratory system. Deposition fractions (DFs) and deposition doses in the head region (DF > 50%) were the highest for PM and BC, for which fine particles (BC, PM1, and PM2.5) were then most easily deposited in the PUL region while coarse particles rarely reach PUL. Children inhaled higher doses of polluted air during active commuting (walking) than passive commuting (private cars, e-bikes), due to longer times of exposure coupled with more active breathing.
Keywords: BC and PM exposure; Children; Commuting to school; Deposition dose.
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