Magnetic structure study of the sawtooth chain antiferromagnet [Formula: see text]

Sci Rep. 2021 Dec 15;11(1):24049. doi: 10.1038/s41598-021-03058-5.

Abstract

A magnetic structure of the sawtooth-chain antiferromagnet [Formula: see text] was investigated by magnetization measurements, single crystalline and powder neutron diffraction experiments, and a further analysis on the Mössbauer spectra. These experiments revealed a nearly collinear antiferromagnetic structure with magnetic moments aligned along the b-axis, indicating dominant antiferromagnetic exchanges between Fe(1)-Fe(2) and Fe(2)-Fe(3) sites. The magnon dispersion relation derived from the linear spin wave approximation suggests the possible flat band nature of magnons.