Plasmonic Nanoparticle Lattice Devices for White-Light Lasing

Adv Mater. 2023 Aug;35(34):e2103262. doi: 10.1002/adma.202103262. Epub 2021 Sep 12.

Abstract

A plasmonic nanolaser architecture that can produce white-light emission is reported. A laser device is designed based on a mixed dye solution used as gain material sandwiched between two aluminum nanoparticle (NP) square lattices of different periodicities. The (±1, 0) and (±1, ±1) band-edge surface lattice resonance (SLR) modes of one NP lattice and the (±1, 0) band-edge mode of the other NP lattice function as nanocavity modes for red, blue, and green lasing respectively. From a single aluminum NP lattice, simultaneous red and blue lasing is realized from a binary dye solution, and the relative intensities of the two colors are controlled by the volume ratio of the dyes. Also, a laser device is constructed by sandwiching dye solutions between two Al NP lattices with different periodicities, which enables red-green and blue-green lasing. With a combination of three dyes as liquid gain, red, green, and blue lasing for a white-light emission profile is realized.

Keywords: lattice plasmons; multi-color lasers; plasmonic nanoparticle lattices; sandwiched devices; surface lattice resonances; white-light lasers.