Global tropospheric ozone responses to reduced NO x emissions linked to the COVID-19 worldwide lockdowns

Sci Adv. 2021 Jun 9;7(24):eabf7460. doi: 10.1126/sciadv.abf7460. Print 2021 Jun.

Abstract

Efforts to stem the transmission of coronavirus disease 2019 (COVID-19) led to rapid, global ancillary reductions in air pollutant emissions. Here, we quantify the impact on tropospheric ozone using a multiconstituent chemical data assimilation system. Anthropogenic NO x emissions dropped by at least 15% globally and 18 to 25% regionally in April and May 2020, which decreased free tropospheric ozone by up to 5 parts per billion, consistent with independent satellite observations. The global total tropospheric ozone burden declined by 6TgO3 (∼2%) in May and June 2020, largely due to emission reductions in Asia and the Americas that were amplified by regionally high ozone production efficiencies (up to 4 TgO3/TgN). Our results show that COVID-19 mitigation left a global atmospheric imprint that altered atmospheric oxidative capacity and climate radiative forcing, providing a test of the efficacy of NO x emissions controls for co-benefiting air quality and climate.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Air Pollutants / analysis*
  • Air Pollution / analysis*
  • Atmosphere / analysis*
  • COVID-19 / epidemiology*
  • COVID-19 / virology
  • Climate
  • Environmental Exposure / analysis*
  • Environmental Monitoring
  • Global Health
  • Humans
  • Nitric Oxide / analysis*
  • Ozone / analysis*
  • SARS-CoV-2 / isolation & purification

Substances

  • Air Pollutants
  • Nitric Oxide
  • Ozone