Deuterogenic Plasmonic Vortices

Nano Lett. 2020 Sep 9;20(9):6774-6779. doi: 10.1021/acs.nanolett.0c02699. Epub 2020 Aug 25.

Abstract

The optical vortex on a chip is of extreme importance for many applications in nanoscience, and as well-known, the chiral metallic nanostructures like plasmonic vortex lenses (PVLs) can produce a spin-dependent plasmonic vortex (PV) which is governed by plasmonic spin-orbit coupling. The well-established nanophotonic theory and various experimental demonstrations all show a single PV mode in one PVL, when the excitation is fixed. Here, counterintuitively, we report the existence of the nontrivial deuterogenic PVs, besides the one predicted previously. We theoretically reveal a general spin-to-orbit coupling and experimentally demonstrate the surprising existence of multiple PVs in a single PVL even when excited by a fixed circularly polarized vortex beam. This work provides a deeper fundamental understanding of the dynamics and the near-field spin-orbit coupling in nanophotonics, which promises to flexibly manipulate the PV for emerging optical vortex-based nanotechnologies and quantum optical applications on a chip.

Keywords: Plasmonic vortex; orbital angular momentum; plasmonic vortex lenses; spin-to-orbit coupling; surface plasmon polaritons.