Riverine deposition pattern of oil-particle aggregates considering the coagulation effect

Sci Total Environ. 2020 Oct 15:739:140371. doi: 10.1016/j.scitotenv.2020.140371. Epub 2020 Jun 20.

Abstract

To understand the heterogeneous behavior of oil-particle aggregates (OPAs) in the riverine environment as well as the uncertainties caused by the coupling effects between their stochastic formation and transportation processes, this study employed the coagulation conceptual formula and random-walk particle tracking model. Through careful inspection using the classic Rouse-Vanoni diagram and existing laboratory observations, a vertical diffusivity scheme and the packing coefficient for an oil-sediment interaction model were determined. The density variations and deposition patterns of hypothetically fully developed OPAs as well as the impact of oil-sediment interactions on the longitudinal distribution of deposited OPAs were then investigated. The results indicate that the formation process of OPAs has a significant effect on their longitudinal deposition. The range of potentially trapped OPAs varied from several to hundreds of times the range of cases that exclude oil-sediment interactions. The deposition diagram proposed in this study visualizes the relationship between the configuration and deposition pattern of OPAs and can assist in determining the most unfavorable scenarios for oil-spill countermeasures. Further refinement and calibration of the model are necessary in the future to provide guidelines for oil spill responses and recovery in riverine environments.

Keywords: Coagulation impact; Lagrangian particle tracking model; Longitudinal deposition; Oil spill; Oil-particle aggregate.