Observation of the hot-phonon effect in monolayer MoS2

Nanotechnology. 2020 Feb 25;31(23):235712. doi: 10.1088/1361-6528/ab79ad. Online ahead of print.

Abstract

Femtosecond transient absorption measurements have been performed to study the pump wavelength- and fluence-dependent hot carrier relaxation dynamics in monolayer MoS2. The relaxation process of the photoinduced carriers monitored within hundreds of femtoseconds after photoexcitation is demonstrated to be achieved through the carrier-phonon scattering mechanism. It is observed that an efficient hot-phonon effect can slow down the relaxation rate by around three times with the injected carrier density changing from 1 × 1012 to 3 × 1013 cm-2. A pronounced increase in the hot carrier relaxation time with decreasing temperature is further detected, which is attributed to the decreased phonon occupancy at lower temperature.