Accumulation rates and chronologies from depth profiles of 210Pbex and 137Cs in sediments of northern Beibu Gulf, South China sea

Jing Guo; Ozeas S Costa Jr; Yinghui Wang; Wuhui Lin; Shaopeng Wang; Bo Zhang; Yefeng Cui; Hao Fu; Linlin Zhang

doi:10.1016/j.jenvrad.2019.106136

Accumulation rates and chronologies from depth profiles of ²¹⁰Pb_ex and ¹³⁷Cs in sediments of northern Beibu Gulf, South China sea

J Environ Radioact. 2020 Mar:213:106136. doi: 10.1016/j.jenvrad.2019.106136. Epub 2019 Dec 15.

Authors

Jing Guo¹, Ozeas S Costa Jr², Yinghui Wang³, Wuhui Lin⁴, Shaopeng Wang⁴, Bo Zhang⁴, Yefeng Cui⁴, Hao Fu⁴, Linlin Zhang⁴

Affiliations

¹ Guangxi Laboratory on the Study of Coral Reefs in the South China Sea, Nanning, 530004, China; School of Marine Sciences, Guangxi University, Nanning, 530004, China; College of Civil Engineering and Architecture, Guangxi University, Nanning, 530004, China; School of Earth Sciences, The Ohio State University at Mansfield, Mansfield, OH, 44906, USA.
² School of Earth Sciences, The Ohio State University at Mansfield, Mansfield, OH, 44906, USA.
³ Guangxi Laboratory on the Study of Coral Reefs in the South China Sea, Nanning, 530004, China; School of Marine Sciences, Guangxi University, Nanning, 530004, China. Electronic address: wyh@gxu.edu.cn.
⁴ Guangxi Laboratory on the Study of Coral Reefs in the South China Sea, Nanning, 530004, China; School of Marine Sciences, Guangxi University, Nanning, 530004, China.

PMID: 31983445
DOI: 10.1016/j.jenvrad.2019.106136

Abstract

Beibu Gulf is a highly dynamic and complex coastal environment that is currently experiencing one of the largest rates of development and urbanization in west China. Little is known about the effects of this increased human activity on coastal sedimentation processes and on the rates of sediment accumulation and the variation of organic materials to the coast. In this study, four sediment cores were collected and applied the ²¹⁰Pb dating method to reconstruct sedimentation rates and historical changes of materials to the northern Beibu Gulf over the past century. Depth profiles of excess ²¹⁰Pb (²¹⁰Pb_ex) showed highest activity values at the surface (28.4-104.0 Bq kg^-1) followed by a linear or exponential decay with depth for all but one study site. ¹³⁷Cs activity ranged between 0.236 and 2.034 Bq kg^-1, and a distinct peak activity - representing the 1963 fallout maximum - was observed at all but one site. Sediment chronologies were determined using the Constant Rate of Supply (CRS) model. Calculated accumulation rates in the studied sites were the lowest in the late 1920s and early 1930s (mass accumulation rate (MAR): 0.06 ± 0.01 g cm^-2 y^-1; sediment accumulation rate (SAR): 0.08 ± 0.01 cm y^-1) and increased gradually until reaching maximum values in the 2010s (MAR: 0.22 ± 0.09 g cm^-2 y^-1; SAR: 0.46 ± 0.32 cm y^-1). Current accumulation rates are up to 800% higher than rates observed in the 1920s, with most of the increase happening after 1970, coinciding with the increasing rate of urbanization and development in the region. The highest increase in SAR over the last century (+877%) was observed in Sanniang Bay, with the lowest rate of increase (+283%) observed in Lianzhou Bay. TOC content in these sediments has also increased over the last 100 years. Current values (0.98-1.28%) are about 170% higher than historical concentrations (before 1970). The positive correlations between TOC and population density and GDP growth in major cities surrounding the gulf, provide further indication that human activities have significantly altered the sedimentary environment in recent decades along the northern Beibu Gulf coast.

Keywords: Beibu Gulf; Geochronology; Radiotracers; Sedimentation rates; South China sea.

MeSH terms

Cesium
China
Environmental Monitoring
Geologic Sediments*
Humans
Lead
Radiation Monitoring*
Water Pollutants, Chemical

Substances

Water Pollutants, Chemical
Cesium
Lead