Fast Cyclization of a Proline-Derived Self-Immolative Spacer Improves the Efficacy of Carbamate Prodrugs

Angew Chem Int Ed Engl. 2020 Mar 2;59(10):4176-4181. doi: 10.1002/anie.201916394. Epub 2020 Jan 22.

Abstract

Self-immolative (SI) spacers are sophisticated chemical constructs designed for molecular delivery or material degradation. We describe herein a (S)-2-(aminomethyl)pyrrolidine SI spacer that is able to release different types of anticancer drugs (possessing either a phenolic or secondary and tertiary hydroxyl groups) through a fast cyclization mechanism involving carbamate cleavage. The high efficiency of drug release obtained with this spacer was found to be beneficial for the in vitro cytotoxic activity of protease-sensitive prodrugs, compared with a commonly used spacer of the same class. These findings expand the repertoire of degradation machineries and are instrumental for the future development of highly efficient delivery platforms.

Keywords: cascade reactions; disassembly; drug delivery; prodrugs; self-immolative spacers.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antineoplastic Agents / chemical synthesis
  • Antineoplastic Agents / chemistry
  • Antineoplastic Agents / pharmacology*
  • Carbamates / chemical synthesis
  • Carbamates / chemistry
  • Carbamates / pharmacology*
  • Cell Line, Tumor
  • Cell Proliferation / drug effects
  • Cyclization
  • Drug Screening Assays, Antitumor
  • Humans
  • Molecular Structure
  • Prodrugs / chemical synthesis
  • Prodrugs / chemistry
  • Prodrugs / pharmacology*
  • Proline / chemical synthesis
  • Proline / chemistry
  • Proline / pharmacology*

Substances

  • Antineoplastic Agents
  • Carbamates
  • Prodrugs
  • Proline