Investigations on chemical composition and natural radioactivity levels from salt water and peloid used in pelotherapy from the Techirghiol Lake, Romania

Environ Geochem Health. 2020 Feb;42(2):513-529. doi: 10.1007/s10653-019-00382-8. Epub 2019 Jul 30.

Abstract

The work presents the historical evolution, objectives, goals, concepts, chemical and radiometric methods, results and conclusions for salt waters and natural peloids used in pelotherapy. This study assesses chemical composition, natural radioactivity concentrations and the radiological hazard in peloid and salt water samples, from ten places in the Techirghiol Lake from Romania. Pelotherapy is a very important procedure, and thus, the materials used for this purpose must be well characterized to guaranty safety use. Concentrations of elements such as Sr, Ba, Mn, Fe, Sb, Zn, Cu, Pb, Ti, Ni, Cr, As have been measured using ICP-OES analytical technique. The natural radionuclides such as 238U, 226Ra, 232Th and 40K have been determined by gamma-ray spectrometry. The average activity concentrations were of 0.48 ± 0.10 Bq/kg for 238U, 0.60 ± 0.10 Bq/kg for 226Ra, 0.30 ± 0.08 Bq/kg for 232Th and 17.5 ± 1.3 Bq/kg for 40K for salt water samples. Also, the mean activity concentrations for peloids were: 5.70 ± 1.00 Bq/kg for 238U, 6.85 ± 1.60 Bq/kg for 232Th, 15.3 ± 3.7 Bq/kg for 226Ra and 95.8 ± 5.5 Bq/kg for 40K. The results from this study contribute to the identification of possible contaminants in the salt water and peloid, and their association with the potential ecological and human health risk. In this context, of using salt water and peloid in a relatively long treatment period, several radiological indices have been calculated, to determine if the radionuclide's content can be also harmful to human health. The assessment indicates that humans are not exposed to concentrations of metal contaminants higher than the international recommended values.

Keywords: Dose assessment; Natural peloid; Natural radioactivity; Pelotherapy; Salt water.

MeSH terms

  • Background Radiation*
  • Gamma Rays
  • Geologic Sediments / analysis
  • Humans
  • Hydrogen-Ion Concentration
  • Lakes / analysis*
  • Lakes / chemistry*
  • Metals / analysis
  • Mud Therapy*
  • Potassium Radioisotopes / analysis
  • Radiation Monitoring / methods
  • Radioisotopes / analysis*
  • Radium / analysis
  • Romania
  • Salinity
  • Spectrometry, Gamma
  • Temperature
  • Thorium / analysis
  • Uranium / analysis

Substances

  • Metals
  • Potassium Radioisotopes
  • Potassium-40
  • Radioisotopes
  • Thorium-232
  • Uranium-238
  • Uranium
  • Thorium
  • Radium-226
  • Radium