Deformable Ionic Polymer Artificial Mechanotransducer with an Interpenetrating Nanofibrillar Network

ACS Appl Mater Interfaces. 2019 Aug 14;11(32):29350-29359. doi: 10.1021/acsami.9b10499. Epub 2019 Aug 1.

Abstract

We demonstrate an ionic polymer artificial mechanotransducer (i-PAM) capable of simultaneously yielding an efficient wide bandwidth and a blocking force to maximize human tactile recognition in soft tactile feedback. The unique methodology in the i-PAM relies on an ionic interpenetrating nanofibrillar network that is formed at the interface of (i) an ionic thermoplastic polyurethane nanofibrillar matrix with an ionic liquid of 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide ([EMIM]+[TFSI]-) and (ii) ionic poly(3,4-ethylenedioxythiophene):poly(styrenesulfonic acid) (PEDOT:PSS) conducting polymer electrodes with dimethyl sulfoxide and [EMIM]+[TFSI]- as additives. The i-PAM-based actuator with the ionic PEDOT:PSS exhibits a stable operation up to 200 Hz at low voltage as well as a blocking force of 0.4 mN, which can be potentially adapted to soft tactile feedback. Furthermore, on the basis of this fast i-PAM, we realized alphabet tactile rendering by using a 3 × 3 i-PAM array stimulated by a dc input of 2 V. We believe that our proposed approach can provide a rational guide to the human-machine soft haptic interface.

Keywords: blocking force; ionic interpenetrating nanofibrillar network; ionic polymer artificial mechanotransducer; soft actuator; soft haptic interface; wide bandwidth.

MeSH terms

  • Bridged Bicyclo Compounds, Heterocyclic / chemistry*
  • Electrodes
  • Humans
  • Imidazoles / chemistry*
  • Nanofibers / chemistry*
  • Polymers / chemistry*
  • Polystyrenes / chemistry*

Substances

  • Bridged Bicyclo Compounds, Heterocyclic
  • Imidazoles
  • Polymers
  • Polystyrenes
  • poly(3,4-ethylene dioxythiophene)
  • polystyrene sulfonic acid
  • 1-ethyl-3-methylimidazolium