Identification of spatial magnetic inhomogeneities by nuclear forward scattering of synchrotron radiation

J Synchrotron Radiat. 2019 Jul 1;26(Pt 4):1310-1315. doi: 10.1107/S1600577519005344. Epub 2019 Jun 12.

Abstract

Spatially confined magnetic inhomogeneities were revealed by measuring nuclear forward scattering time spectra on the same sample in two different geometric arrangements. They differ by 180° rotation of the sample around one of the polarization axes. A basic theoretical description of this phenomenon and its relation to a spatial distribution of nuclei featuring different magnetic moments is provided. From an experimental point of view, the violation of rotational invariance was observed for an inhomogeneous Fe81Mo8Cu1B10 metallic glass. The development of magnetic inhomogeneities and their relation to the evolution of time spectra was studied during thermal annealing.

Keywords: Mössbauer spectroscopy; magnetic inhomogeneities; metallic glasses; nuclear forward scattering; rotational invariance.