Sawtooth Torque in Anisotropic j_{eff}=1/2 Magnets: Application to α-RuCl_{3}

Phys Rev Lett. 2019 May 17;122(19):197202. doi: 10.1103/PhysRevLett.122.197202.

Abstract

The so-called "Kitaev candidate" materials based on 4d^{5} and 5d^{5} metals have recently emerged as magnetic systems displaying strongly anisotropic exchange interactions reminiscent of the Kitaev's honeycomb model. Recently, these materials have been shown to commonly display a distinct sawtooth angular dependence of the magnetic torque over a wide range of magnetic fields. While higher order chiral spin interactions have been considered as a source of this observation, we show here that bilinear anisotropic interactions and/or g anisotropy are each sufficient to explain the observed torque response, which may be distinguished on the basis of high-field measurements. These findings unify the understanding of magnetic torque experiments in a variety of Kitaev candidate materials.