A Local Study of the Transport Mechanisms in MoS2 Layers for Magnetic Tunnel Junctions

ACS Appl Mater Interfaces. 2018 Sep 12;10(36):30017-30021. doi: 10.1021/acsami.8b08853. Epub 2018 Aug 27.

Abstract

MoS2-based vertical spintronic devices have attracted an increasing interest thanks to theoretical predictions of large magnetoresistance signals. However, experimental performances are still far from expectations. Here, we carry out the local electrical characterization of thin MoS2 flakes in a Co/Al2O3/MoS2 structure through conductive tip AFM measurements. We show that thin MoS2 presents a metallic behavior with a strong lateral transport contribution that hinders the direct tunnelling through thin layers. Indeed, no resistance dependence is observed with the flake thickness. These findings reveal a spin depolarization source in the MoS2-based spin valves, thus pointing to possible solutions to improve their spintronic properties.

Keywords: 2D materials; MoS2; conductive tip AFM; magnetic tunnel junctions; spin valves; spintronics; vertical transport.