Theoretical spin-wave dispersions in the antiferromagnetic phase AF1 of MnWO4 based on the polar atomistic model in P2

J Phys Condens Matter. 2018 Jul 25;30(29):295401. doi: 10.1088/1361-648X/aaca67. Epub 2018 Jun 5.

Abstract

The spin wave dispersions of the low temperature antiferromagnetic phase (AF1) MnWO4 have been numerically calculated based on the recently reported non-collinear spin configuration with two different canting angles. A Heisenberg model with competing magnetic exchange couplings and single-ion anisotropy terms could properly describe the spin wave excitations, including the newly observed low-lying energy excitation mode [Formula: see text] meV appearing at the magnetic zone centre. The spin wave dispersion and intensities are highly sensitive to two differently aligned spin-canting sublattices in the AF1 model. Thus this study reinsures the otherwise hardly provable hidden polar character in MnWO4.