Engineered Sulfur-Resistant Catalyst System with an Assisted Regeneration Strategy for Lean-Burn Methane Combustion

ChemCatChem. 2018 Apr 9;10(7):1556-1560. doi: 10.1002/cctc.201701884. Epub 2018 Feb 27.

Abstract

Catalytic combustion of methane, the main component of natural gas, is a challenge under lean-burn conditions and at low temperatures owing to sulfur poisoning of the Pd-rich catalyst. This paper introduces a more sulfur-resistant catalyst system that can be regenerated during operation. The developed catalyst system lowers the barrier that has restrained the use of liquefied natural gas as a fuel in energy production.

Keywords: emission conversion; green chemistry; low emissions; natural gas; sulfur.