Laser-induced changes of nonlinear electronic transport properties in La0.75Ba0.25MnO3 and (La0.6Pr0.4)0.67Ca0.33MnO3

J Phys Condens Matter. 2018 Jan 31;30(4):045701. doi: 10.1088/1361-648X/aa9fa1.

Abstract

We report photoinduced effects in nonlinear third harmonic ac electric transport-which is a measure for the density of correlated polarons-in thin films of [Formula: see text] (LBMO) and [Formula: see text] (LPCMO) manganites. Both materials show an enhancement of third harmonic voltage in the vicinity of the metal-to-insulator transition, indicating strong electron-lattice correlations within a phase-separated state. Relatively low laser excitation with a pulse fluence of [Formula: see text] leads to an increase (decrease) in nonlinearity in LBMO (LPCMO). With a high pulse fluence of 8mJ cm-2, we were also able to suppress the correlations in LBMO, which is accompanied by a decrease of third harmonic voltage by [Formula: see text] in our time-averaging measurement technique.