Measurement of Nanoplasmonic Field Enhancement with Ultrafast Photoemission

Nano Lett. 2017 Feb 8;17(2):1181-1186. doi: 10.1021/acs.nanolett.6b04893. Epub 2017 Jan 20.

Abstract

Probing nanooptical near-fields is a major challenge in plasmonics. Here, we demonstrate an experimental method utilizing ultrafast photoemission from plasmonic nanostructures that is capable of probing the maximum nanoplasmonic field enhancement in any metallic surface environment. Directly measured field enhancement values for various samples are in good agreement with detailed finite-difference time-domain simulations. These results establish ultrafast plasmonic photoelectrons as versatile probes for nanoplasmonic near-fields.

Keywords: Nanoplasmonics; femtosecond laser pulses; field enhancement; photoelectrons; ultrafast interactions.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Electromagnetic Fields
  • Fluorescence
  • Gold / chemistry
  • Kinetics
  • Lasers
  • Metal Nanoparticles / chemistry*
  • Photoelectron Spectroscopy
  • Silver / chemistry
  • Surface Properties

Substances

  • Silver
  • Gold