Room Temperature Semiconductor-Metal Transition of MoTe2 Thin Films Engineered by Strain

Nano Lett. 2016 Jan 13;16(1):188-93. doi: 10.1021/acs.nanolett.5b03481. Epub 2015 Dec 31.

Abstract

We demonstrate a room temperature semiconductor-metal transition in thin film MoTe2 engineered by strain. Reduction of the 2H-1T' phase transition temperature of MoTe2 to room temperature was realized by introducing a tensile strain of 0.2%. The observed first-order SM transition improved conductance ∼10 000 times and was made possible by an unusually large temperature-stress coefficient, which results from a large volume change and small latent heat. The demonstrated strain-modulation of the phase transition temperature is expected to be compatible with other TMDs enabling the 2D electronics utilizing polymorphism of TMDs along with the established materials.

Keywords: MoTe2; Strain; modulation; phase transition; semiconductor-metal transition.

Publication types

  • Research Support, Non-U.S. Gov't