Southwest intrusion of 134Cs and 137Cs derived from the Fukushima Dai-ichi nuclear power plant accident in the Western North Pacific

Environ Sci Technol. 2014 Mar 18;48(6):3120-7. doi: 10.1021/es403686v. Epub 2014 Mar 7.

Abstract

Enormous quantities of radionuclides were released into the ocean via both atmospheric deposition and direct release as a result of the Fukushima Dai-ichi Nuclear Power Plant (FNPP) accident. This study discusses the southward dispersion of FNPP-derived radioactive cesium (Cs) in subsurface waters. The southernmost point where we found the FNPP-derived (134)Cs (1.5-6.8 Bq m(-3)) was 18 °N, 135 °E, in September 2012. The potential density at the subsurface peaks of (134)Cs (100-500 m) and the increased water column inventories of (137)Cs between 0 and 500 m after the winter of 2011-2012 suggested that the main water mass containing FNPP-derived radioactive Cs was the North Pacific Subtropical Mode Water (NPSTMW), formed as a result of winter convection. We estimated the amount of (134)Cs in core waters of the western part of the NPSTMW to be 0.99 PBq (decay-corrected on 11 March 2011). This accounts for 9.0% of the (134)Cs released from the FNPP, with our estimation revealing that a considerable amount of FNPP-derived radioactive Cs has been transported to the subtropical region by the formation and circulation of the mode water.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cesium Radioisotopes / analysis*
  • Fukushima Nuclear Accident*
  • Japan
  • Nuclear Power Plants*
  • Pacific Ocean
  • Radiation Monitoring
  • Water Pollutants, Radioactive / analysis*

Substances

  • Cesium Radioisotopes
  • Water Pollutants, Radioactive