Evidence for a rapid release of carbon at the Paleocene-Eocene thermal maximum

Proc Natl Acad Sci U S A. 2013 Oct 1;110(40):15908-13. doi: 10.1073/pnas.1309188110. Epub 2013 Sep 16.

Abstract

The Paleocene/Eocene thermal maximum (PETM) and associated carbon isotope excursion (CIE) are often touted as the best geologic analog for the current anthropogenic rise in pCO2. However, a causal mechanism for the PETM CIE remains unidentified because of large uncertainties in the duration of the CIE's onset. Here, we report on a sequence of rhythmic sedimentary couplets comprising the Paleocene/Eocene Marlboro Clay (Salisbury Embayment). These couplets have corresponding δ(18)O cycles that imply a climatic origin. Seasonal insolation is the only regular climate cycle that can plausibly account for δ(18)O amplitudes and layer counts. High-resolution stable isotope records show 3.5‰ δ(13)C decrease over 13 couplets defining the CIE onset, which requires a large, instantaneous release of (13)C-depleted carbon. During the CIE, a clear δ(13)C gradient developed on the shelf with the largest excursions in shallowest waters, indicating atmospheric δ(13)C decreased by ~20‰. Our observations and revised release rate are consistent with an atmospheric perturbation of 3,000-gigatons of carbon (GtC).

Keywords: carbon cycle; climate change.

Publication types

  • Historical Article
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Atmosphere / analysis*
  • Carbon Isotopes / analysis*
  • Climate Change*
  • Geologic Sediments / analysis*
  • Geology / methods*
  • History, Ancient
  • Oceans and Seas

Substances

  • Carbon Isotopes