Models for integrated and differential scattering optical properties of encapsulated light absorbing carbon aggregates

Opt Express. 2013 Apr 8;21(7):7974-93. doi: 10.1364/OE.21.007974.

Abstract

Optical properties of light absorbing carbon (LAC) aggregates encapsulated in a shell of sulfate are computed for realistic model geometries based on field measurements. Computations are performed for wavelengths from the UV-C to the mid-IR. Both climate- and remote sensing-relevant optical properties are considered. The results are compared to commonly used simplified model geometries, none of which gives a realistic representation of the distribution of the LAC mass within the host material and, as a consequence, fail to predict the optical properties accurately. A new core-gray shell model is introduced, which accurately reproduces the size- and wavelength dependence of the integrated and differential optical properties.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Absorption
  • Carbon / chemistry*
  • Carbon / radiation effects*
  • Light*
  • Models, Chemical*
  • Scattering, Radiation
  • Systems Integration

Substances

  • Carbon