First-principles calculations of quasiparticle excitations of open-shell condensed matter systems

Phys Rev Lett. 2012 Jul 20;109(3):036406. doi: 10.1103/PhysRevLett.109.036406. Epub 2012 Jul 20.

Abstract

We develop a Green's function approach to quasiparticle excitations of open-shell systems within the GW approximation. It is shown that accurate calculations of the characteristic multiplet structure require a precise knowledge of the self-energy and, in particular, its poles. We achieve this by constructing the self-energy from appropriately chosen mean-field theories on a fine frequency grid. We apply our method to a two-site Hubbard model, several molecules, and the negatively charged nitrogen-vacancy defect in diamond and obtain good agreement with experiment and other high-level theories.