High-energy, broadly tunable, narrow-bandwidth mid-infrared optical parametric system pumped by quasi-phase-matched devices

Opt Lett. 2008 Aug 1;33(15):1699-701. doi: 10.1364/ol.33.001699.

Abstract

We have developed a tunable, narrow-bandwidth (<2 cm(-1)) mid-infrared (MIR) optical parametric system with a large-aperture periodically poled Mg-doped LiNbO(3) (LA-PPMgLN)-based high-energy pump source. The system has a continuously tunable tuning range from 4.6 to 11.2 mum and produces a maximum output energy of 2.0 mJ at 5.1 mum. Practical use of the MIR source is demonstrated by MIR-UV double-resonance spectroscopy of jet-cooled acetanilide.