Small atomic displacements recorded in bismuth by the optical reflectivity of femtosecond laser-pulse excitations

Phys Rev Lett. 2008 Jan 18;100(2):027404. doi: 10.1103/PhysRevLett.100.027404. Epub 2008 Jan 18.

Abstract

Subtle atomic motion in a Bi crystal excited by a 35 fs-laser pulse has been recovered from the transient reflectivity of an optical probe measured with an accuracy of 10(-5). Analysis shows that a novel effect reported here-an initial negative drop in reflectivity-relates to a delicate coherent displacement of atoms by the polarization force during the pulse. We also show that reflectivity oscillations with a frequency coinciding with that of cold Bi are related to optical phonons excited by the electron temperature gradient through electron-phonon coupling.