Geometry of dynamically available empty space is the key to near-arrest dynamics

Phys Rev E Stat Nonlin Soft Matter Phys. 2005 Aug;72(2 Pt 1):021401. doi: 10.1103/PhysRevE.72.021401. Epub 2005 Aug 3.

Abstract

We study several examples of kinetically constrained lattice models using dynamically accessible volume as an order parameter. Thereby we identify two distinct regimes exhibiting dynamical slowing, with a sharp threshold between them. These regimes are identified both by a new response function in dynamically available volume, as well as directly in the dynamics. Results for the self-diffusion constant in terms of the connected hole density are presented, and some evidence is given for scaling in the limit of dynamical arrest.